Such low-level sound control is unlikely to be supported by the .Net framework, so you will probably need to look into using the Win32 API - specifically various multimedia functions. However, manipulating the amplitudes of different frequency bands may still not be supported, meaning youll have to write the DSP routines yourself - a very daunting task if youre not well grounded in DSP.
I have written quite a few DSP applications myself, and I would recommend using C++ to write your underlying DSP routines and use VB.Net only for the GUI.
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